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《Journal of the European Ceramic Society》2020,40(15):5475-5482
The lead-free Ba0.53Sr0.47TiO3 (BST) thin films buffered with La0.67Sr0.33MnO3 (LSMO) bottom electrode of different thicknesses were fabricated by pulsed laser deposition method on a (001) SrTiO3 substrate. It was found that the roughness of electrode decreases and substrate stress relaxes gradually with the increase of LSMO thickness, which is beneficial for weakening local high electric field and achieving higher Eb. Therefore, the recoverable energy density (Wrec) of BST films can be greatly improved up to 67.3 %, that is, from 30.6 J/cm3 for the LSMO thickness of 30 nm up to 51.2 J/cm3 for the LSMO thickness of 140 nm after optimizing the LSMO thickness. Furthermore, the thin film capacitor with a 140 nm LSMO bottom electrode shows an outstanding thermal stability from 20 °C to 160 °C and superior fatigue resistance after 108 electrical cycles with only a slightly decrease of Wrec below 1.6 % and 3.7 %, respectively. Our work demonstrates that optimizing bottom electrodes thickness is a promising way for enhancing energy storage properties of thin-film capacitors. 相似文献
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《Ceramics International》2020,46(14):22452-22459
Relaxor ferroelectrics have attracted much attention as electric energy storage materials for intermittent energy storage because of their high saturated polarization, near-zero remnant polarizations, and considerable dielectric breakdown strength (BDS). Despite the numerous efforts, the dielectric energy storage performance of relaxor ferroelectric ceramics is incomplete or unsatisfactory. The enhancement of recoverable energy storage density Wrec usually accompanies with the sacrifice of discharge-to-charge energy efficiency η; therefore, it is an important issue to achieve high recoverable Wrec and large efficiency η simultaneously. In this work, the (1-x)BaTiO3-xBi(Zn1/2Zr1/2)O3 (abbreviated as BT-100xBZZ, 0 ≤ x ≤ 0.20) ferroelectric ceramics were prepared using the conventional solid-state reaction method. The phase structure, microstructural morphology, dielectric and ferroelectric properties, relaxation behaviors, and energy storage properties of BT-BZZ ceramics were investigated in detail. X-ray powder diffraction, dielectric spectra, and ferroelectric properties confirm the transformation of tetragonal phase for normal ferroelectrics (BT) to pseudo-cubic phase for relaxor ferroelectrics (BT-8BZZ). A high recoverable energy storage density Wrec of 2.47 J/cm3 and a large energy efficiency η of 94.4% are simultaneously achieved in the composition of BT-12BZZ, which presents typical weakly coupled relaxor ferroelectric characteristics, with an activation energy Ea of 0.21 eV and a freezing temperature Tf of 139.7 K. Such excellent energy storage performance suggests that relaxor ferroelectric BT-12BZZ ceramics are promising dielectric energy storage materials for high-power pulsed capacitors. 相似文献
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The intermittent wind power in isolated hybrid distributed generation (IHDG) may cause serious problems associated with frequency (f) and power (P) fluctuation. Energy storage devices such as battery, super capacitor, and superconducting magnetic energy storage (SMES) may be used to reduce these fluctuations associated with f and P. This paper presents a study of IHDG power system for improving both f and P deviation profiles with the help of SMES. The studied IHDG power system is consisted of wind turbine generator and diesel engine generator. Both f and P control problems of the studied power system model are addressed in presence or absence of SMES. Fuzzy logic based proportional–integral–derivative (PID) controller with SMES is used for the purpose of minimization of f and P deviations. The different tunable parameters of the PID controller and those of the SMES are tuned by a novel quasi-oppositional harmony search algorithm. Performance study of the IHDG power system model is carried out under different perturbation conditions. The results demonstrate minimum f and P deviations may be achieved by using the proposed fuzzy logic based PID controller along with SMES. 相似文献
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针对云冈矿12#煤层8820、8822采空区出现CO泄漏事件,采用粉煤灰填充,构筑木板墙充填粉煤灰,配以墙体周边注马丽散堵漏;采用灌浆泵进行地面黄土灌浆,实施采空区灭火。通过对采空区自然发火进行综合治理,取得了良好效果,消除了自然发火隐患。 相似文献
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针对煤矿“双重预防体系”如何落地生根问题,结合陈四楼煤矿在风险分级管控和隐患排查治理方面的实用方法和“双重预防体系”的建设经验,深入研究了“双重预防体系”的相关标准、风险隐患事故之间的关系及其各自的产生和发展机理、安全风险的有关辨识评估方法、事故隐患的排查和治理方法,分析了传统安全管理模式与“双重预防体系”的新型安全管理模式的差别,总结出了“123456双重预防体系”这个囊括了事前安全风险辨识、事中隐患排查治理、事后安全现状评估的创新成果,实现了“事前、事中、事后”的全过程控制,对夯实煤矿安全管理根基、促进矿井平稳有序发展发挥着越来越重要的作用,为煤炭行业“双重预防体系”的落地生根提供了借鉴和参考。 相似文献
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Goat milk has specific chemical composition and physical properties. The purpose of this study was to investigate the change of milk quality and emulsion stability during 60 d frozen storage. Milk sample was taken from three Ettawah Crossedbred goats that were divided into three groups. Samples were frozen and stored for 0, 30 and 60 days. At the end of each storage periode, milk sample was thawed in the refrigerator and analyzed for total number of bacteria, chemical (acidity, pH, free fatty acids), physical (alcohol test, clot on boiling test) quality, and emulsion stability. The microbiological and chemical data were analyzed statistically using one way ANOVA, whereas physical quality and emulsion stabilty were expressed qualitatively. There were no change in the total bacteria, acidity, pH and free fatty acid (FFA) of milk during storage, whereas the assessment by 70% alcohol showed positive since 0 d. Emulsions stability changed after 30 d of storage. While, the clot on boiling (COB) test of milk was positive at 60 d of storage. Recommendation is frozen storage of goat milk should not longer than 30 d. 相似文献